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This work presents a novel method for upcycling polyethylene terephthalate (PET) waste into sustainable vitrimer materials. By combining bio-based crosslinkers with our PET-based macromonomer, we developed dynamically bonded plastics that are renewably sourced.

With the ever-increasing problem of plastic waste, several avenues to decrease plastic use and manage waste introduced by disposable plastic products have arisen.

Carbon capture from air typically requires large amounts of solvent and sorbent that are energetically costly to regenerate. It also suffers from degradation, is environmentally unsustainable, and very expensive.